Major Chemistry B.Sc.III ( Semester V) Spectral analysis (Problems based on Mass Spectroscopy)

 


 Major Chemistry B.Sc.III ( Semester V)

Name of paper- Spectral analysis

CHE/DSC/T/301 

Problems based on Mass Spectroscopy

Exercise 1.Predict the relative abundance of the parent ion in the case of: (a) Propane (b) n-Pentane

Solution

The relative abundance of the propane molecular ion is greater than that of n-pentane. The abundance of the molecular ion peak can be increased with respect to the abundance of fragment ions by recording the spectrum at low ionisation potential, i.e., by bombarding the sample with low-energy electrons.

Exercise 2. Calculate molecular formula of a compound with molecular mass 94 amu.

Solution. n = 7 and r =3

Mass spectroscopy problem figure

The base formula is C7H10 The index of hydrogen deficiency or DBE = (7-3+2)/2 = 3

Exercise3. Identify the compound having m/e values at 72, 71, 44 (100%), 43, 29 etc.

Solution. Here a signal at 44 (100%) is due to McLafferty rearrangement ion. Clearly, it is a straight chain aldehyde as M⁺ peak at 72 also accompanies M⁺ − 1 peak at 71. Hence formula of the compound is CH₃CH₂CH₂CHO.

Exercise 4. Determine the molecular formula of the compound from the following mass spectrum

Mass spectroscopy problem figure

Solution. Since the pair of peaks are of equal intensity, it is a bromo compound. Two isotopes of bromine are Br⁷⁹ and Br⁸¹. The pair on the extreme right is due to M⁺ and (M⁺ + 2) peaks. The spectrum corresponds to the molecular formula C₂H₅Br.

Exercise5. Explain its fragmentation pattern of pentanal.

Solution: Fragmentation pattern of pentanal is as follows

Mass spectroscopy problem figure

Exercise6. Explain its fragmentation pattern of 3- pentanone

Solution: Fragmentation pattern of 3-pentanone is as follows

Mass spectroscopy problem figure

Exercise7. Predict different peaks in the mass spectrum of ethyl chloride.

Solution. Peaks are seen at:

64 (M⁺)

66 (M⁺ + 2) (intensity ratio 3 : 1)

29 (Base peak)

The loss of Cl• (chlorine radical) occurs.

Exercise8. Explain its fragmentation pattern of 1-bromohexane.

Solution: Various fragmentation modes of 1-bromohexane shown below.

Mass spectroscopy problem figure

Exercise9. Explain its fragmentation pattern of 1-butanol.

Solution: Various fragmentation modes of 1-butanol shown below.

Mass spectroscopy problem figure

Exercise10.The following figure shows the mass spectrum of a saturated hydrocarbon (containing only carbon and hydrogen with only single bonds between carbons, not double bonds).Draw five different structures that would have the molecular weight of this compound. Choose three smaller m/z values from the spectrum and draw one structure for each of them. Note that these fragments will not have complete Lewis structures.

Mass spectroscopy problem figure


Solution: Molecular Weight = 114, which cooresponds to a C8H18 hydrocarbon. There is the possibility of 18 isomers, but here are a few isomers:

Mass spectroscopy problem figure
Mass spectroscopy problem figure

Exercise11. What are the masses of all the components in the following fragmentations?

Solution: The first undergoes an alpha cleavage. The second undergoes a dehydration. The final one goes througha  McLafferty rearrangement.
Mass spectroscopy problem figure

Exercise 12: 5-Chloro-2-pentanone has the mass spectrum shown. Which peak represents the M+? Which is the base peak? Why is there a peak at 122? Explain what the fragment for the base peak would be.

Mass spectroscopy problem figure

Solution: M+ = 120

Base peak = 43

The m/z peak at 122 is the M + 2 peak. It occurs because chlorine has two isotopes 35C and 37C in a 3:1 ratio. The m/z = 43 occurs due to the alpha cleavage. The acylium ion has an m/z of 43. This fragment is particularly stable due to resonance.

Mass spectroscopy problem figure

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